Correlated high spatial resolution elemental and isotopic characterization of Wild 2 cometary samples.

Stadermann F. J., Floss C., and Bose M. (2007)
Lunar Planet. Sci. XXXVIII, Abstract #1334.


ABSTRACT

NASA's Stardust mission was successfully completed with the return of the first bona fide cometary samples for laboratory studies, and the preliminary examination yielded some unexpected results about the composition and origin of cometary matter. From an isotopic point of view, the most important findings were (a) the fact that the majority of the samples are isotopically normal, (b) the observation of CAI-like (Ca-Al-rich inclusions) material with a 16O-enriched composition similar to what has been seen in meteorites, (c) the detection of D and N anomalies indicative of an interstellar heritage of some organics, and (d) the discovery of one - but only one - incontrovertible circumstellar grain.

While isotopic data alone can provide important clues about a given sample, essential insight can frequently only be gained by combining isotopic information with spatially correlated elemental and mineralogical data. Such a complementary analytical approach is especially mandatory in cases of rare or valuable samples such as the cometary matter from Wild 2. For samples that are heterogeneous on a submicrometer scale, the NanoSIMS is the optimal tool for a detailed isotopic characterization. Transmission electron microscopy (TEM) is the technique of choice for detailed mineralogical information and as such provides an ideal complement to the NanoSIMS. Many types of samples, however, are not electrontransparent and thus not immediately accessible for TEM measurements. In such cases, however, it is still possible to use Auger spectroscopy for elemental imaging on a spatial scale of tens of nanometers, well below the working range of EDX characterization. Here we describe the application of complementary high resolution isotopic and elemental imaging for the analysis of cometary samples.


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